杩戞棩锛屼腑鍥界瀛︽妧鏈ぇ瀛︽暀鎺堟浘鏉板洟闃熷湪浣庢俯鐢茬兎姘у寲鍒朵箼閰哥爺绌舵柟闈㈠彇寰楄繘灞曘€傝鐮旂┒鎶ラ亾浜嗗垎瀛愮瓫璐熻浇鐨勯噾-閾佸弻閲戝睘鍌寲鍓傘€傝繖涓€鍌寲鍓傚湪姘翠腑浠ユ哀姘斾负姘у寲鍓傦紝骞跺湪涓€姘у寲纰冲瓨鍦ㄤ笅灏嗙敳鐑锋哀鍖栦负涔欓吀銆傚叿浣撹€岃█锛岄噾绾崇背绮掑瓙鍌寲涓€姘у寲纰筹紝姘ф皵鍜屾按鐢熸垚娲绘€х緹鍩虹墿绉嶏紝鑰屽師瀛愮骇鍒嗘暎鐨勯搧鐗╃淇冭繘缇熷熀浠嬪鐨勭敳鐑锋哀鍖栧拰纰?纰冲伓鑱旇繃绋嬶紝浠庤€岀敓鎴愪箼閰搞€傚湪120鈩冨弽搴?灏忔椂鐨勬潯浠朵笅锛屽垎瀛愮瓫璐熻浇鐨勯噾-閾佸弻閲戝睘鍌寲鍓傚疄鐜颁簡5.7姣懇灏旀瘡鍏嬬殑涔欓吀鏀剁巼锛屾恫鐩镐骇鐗╀腑涔欓吀閫夋嫨鎬ц揪鍒?2%銆傚悓鏃讹紝璇ュ偓鍖栧墏鍦?0鈩冧緷鐒惰〃鐜板嚭娲绘€с€傚洜姝わ紝缇熷熀浠嬪鐨勭瓥鐣ュ湪涔欑兎姘у寲鍒朵笝閰稿拰涓欑兎姘у寲鍒朵竵閰镐腑鍏锋湁搴旂敤鍓嶆櫙銆侟/p>
鐢变簬鐢茬兎鐨勫寲瀛︽儼鎬у拰姘ф皵鐨勪綆娲绘€э紝鍦ㄤ綆娓╀笅浠ユ哀姘旀哀鍖栫敳鐑峰埗涔欓吀闈复鎸戞垬銆傝鐮旂┒鍦ㄧ敳鐑峰拰姘ф皵浣撶郴鍐呭紩鍏ヤ竴姘у寲纰充负涔欓吀鍚堟垚鎻愪緵浜嗘柊璺嚎銆傚湪璇ュ弽搴斾腑锛屼竴姘у寲纰充綔涓鸿繕鍘熷墏銆侀厤浣撳拰鍙嶅簲鐗╃殑浣滅敤宸茶璁よ瘑銆傜劧鑰岋紝杩欎簺鍌寲鍓傞€氬父闇€鍦?50鈩冨乏鍙冲疄鐜扮敳鐑锋哀鍖栧埗涔欓吀锛屽湪杈冧綆娓╁害鏃跺嚑涔庢病鏈変箼閰哥敓鎴愩€傜洰鍓嶏紝鍦ㄤ綆娓╀笅灏嗙敳鐑锋哀鍖栦负涔欓吀閫氬父渚濊禆浜庡己姘у寲鍓傜殑浣跨敤锛屽杩囨哀鍖栨阿鎴栬繃纭吀閽句笌涓夋盁涔欓吀鐨勬贩鍚堢墿銆傚洜姝わ紝鎺㈣涓€姘у寲纰冲強婧跺墏姘寸殑鍏朵粬浣滅敤浠ュ疄鐜颁綆娓╀笅姘ф皵姘у寲鐢茬兎鍒朵箼閰稿叿鏈夐噸瑕佹剰涔夈€侟/p>
鍒嗗瓙绛涜礋杞界殑閲?閾佸弻閲戝睘鍌寲鍓傚湪60鈩冭嚦120鈩冧笅瀹炵幇浜嗙敳鐑锋哀鍖栧埗涔欓吀锛屼笖璇ュ偓鍖栧墏鑳藉琚娆″惊鐜娇鐢ㄣ€傚悓浣嶇礌鏍囪瀹為獙銆佹崟鑾峰疄楠屻€佸垎娈靛疄楠屻€侀『纾佸叡鎸€侀珮鍒嗚鲸璐ㄨ氨鍜屽師浣嶆极鍙嶅皠绾㈠缁撴灉琛ㄦ槑锛屼竴姘у寲纰冲湪姘村瓨鍦ㄤ笅杈呭姪姘ф皵娲诲寲涓烘椿鎬х緹鍩虹墿绉嶃€傚悓鏃讹紝闅忓嵆鐢熸垚鐨勬椿鎬х緹鍩虹墿绉嶄粙瀵肩敳鐑锋哀鍖栧苟涓庝竴姘у寲纰冲彂鐢熺⒊-纰冲伓鑱旂敓鎴愪箼閰搞€侟/p>
璇ョ爺绌朵负浣庢俯涓嬪皢鐢茬兎姘у寲涓轰箼閰告彁渚涗簡楂樻晥鍌寲鍓傦紝骞舵繁鍖栦簡绉戝瀹跺姘у寲鍓備綔鐢ㄧ殑璁ょ煡銆傜浉鍏崇爺绌舵垚鏋滀互Highly Selective Synthesis of Acetic Acid from Hydroxyl鈥怣ediated Oxidation of Methane at Low Temperatures涓洪锛屽彂琛ㄥ湪銆婂痉鍥藉簲鐢ㄥ寲瀛︺€嬩笂銆傜爺绌跺伐浣滃緱鍒扮瀛︽妧鏈儴銆佸浗瀹惰嚜鐒剁瀛﹀熀閲戝鍛樹細銆佷腑鍥界瀛﹂櫌绛夌殑鏀寔銆侟/p>
璁烘枃閾炬帴銆恏ttps://onlinelibrary.wiley.com/doi/10.1002/anie.202412995銆慄/p>
浣庢俯鐢茬兎姘у寲鍒朵箼閰哥殑鍙嶅簲鎬ц兘